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  • Authors: H. E. Bass; Steven D. Hottman;
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  • Authors: Robert D. Coombe; George C. Pimentel;
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  • Authors: Donald Rapp;
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  • Authors: Jon G. Moehlmann; J. D. McDonald;
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  • Authors: Charles L. Beckel;
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  • Authors: V. Robert Stull; Philip J. Wyatt; Gilbert N. Plass;

    The vibrational energy levels of the eight most abundant isotopic species of carbon dioxide have been calculated. Over 1800 energy levels are given for each isotope. The calculations included terms to the third order in the vibrational quantum numbers and took account of the Fermi resonance. The matrices were diagonalized by an eigenvalue routine of great accuracy.

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  • Authors: D. F. Kelley; B. D. Barton; L. Zalotai; B. S. Rabinovitch;
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  • Authors: H. K. Shin;

    The vibrational de-excitation process H2O(010)+H2O(000) →H2O(000)+H2O(000) has been investigated to determine its temperature dependence at low temperatures recognizing the manifestation of strong molecular attraction at such temperatures and considering the transfer of vibrational energy to both the oscillatory motion of weakly-bound complexes and the free rotational motion. The model predicts large values of the de-excitation probability with a strong negative temperature dependence in 200–400 °K; the probability varies from 0.46 at 200 °K to 0.16 at 400 °K.

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  • Authors: Joseph T. Vanderslice; Stanley Weissman;

    The Schwartz—Slawsky—Herzfeld (SSH) theory of vibrational relaxation times assumes that the most effective relative kinetic energy for causing a vibrational transition is much greater than the quantum of energy transferred. For many actual cases, this assumption is not a good one. However, it appears that this approximation can be eliminated with little change in the resulting equations. The force law for N2, determined with the modified equations from the experimental data on relaxation times, does not differ appreciably from previous results.

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  • Authors: D. Rosen; J. Coughlin; R. L. Taylor;

    Measurements of the rate of vibrational energy transfer occuring in H2/HCl molecular system at temperatures 800–2000° K are reported. (AIP)

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  • Authors: H. E. Bass; Steven D. Hottman;
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  • Authors: Robert D. Coombe; George C. Pimentel;
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    46
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  • Authors: Donald Rapp;
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  • Authors: Jon G. Moehlmann; J. D. McDonald;
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  • Authors: Charles L. Beckel;
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  • Authors: V. Robert Stull; Philip J. Wyatt; Gilbert N. Plass;

    The vibrational energy levels of the eight most abundant isotopic species of carbon dioxide have been calculated. Over 1800 energy levels are given for each isotope. The calculations included terms to the third order in the vibrational quantum numbers and took account of the Fermi resonance. The matrices were diagonalized by an eigenvalue routine of great accuracy.

    addClaim

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    31
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  • Authors: D. F. Kelley; B. D. Barton; L. Zalotai; B. S. Rabinovitch;
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  • Authors: H. K. Shin;

    The vibrational de-excitation process H2O(010)+H2O(000) →H2O(000)+H2O(000) has been investigated to determine its temperature dependence at low temperatures recognizing the manifestation of strong molecular attraction at such temperatures and considering the transfer of vibrational energy to both the oscillatory motion of weakly-bound complexes and the free rotational motion. The model predicts large values of the de-excitation probability with a strong negative temperature dependence in 200–400 °K; the probability varies from 0.46 at 200 °K to 0.16 at 400 °K.

    addClaim

    This Research product is the result of merged Research products in OpenAIRE.

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    16
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  • Authors: Joseph T. Vanderslice; Stanley Weissman;

    The Schwartz—Slawsky—Herzfeld (SSH) theory of vibrational relaxation times assumes that the most effective relative kinetic energy for causing a vibrational transition is much greater than the quantum of energy transferred. For many actual cases, this assumption is not a good one. However, it appears that this approximation can be eliminated with little change in the resulting equations. The force law for N2, determined with the modified equations from the experimental data on relaxation times, does not differ appreciably from previous results.

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  • Authors: D. Rosen; J. Coughlin; R. L. Taylor;

    Measurements of the rate of vibrational energy transfer occuring in H2/HCl molecular system at temperatures 800–2000° K are reported. (AIP)

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